Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes (2024)

Li, L., Duan, H., Li, J., Zhang, L., Deng, Y., & Chen, G. (2021). Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes. Advanced Energy Materials, 11(28), Article 2003154. https://doi.org/10.1002/aenm.202003154

Li, Liansheng ; Duan, Huanhuan ; Li, Jia et al. / Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes. In: Advanced Energy Materials. 2021 ; Vol. 11, No. 28.

@article{316c3c5ca6394e71ae878ee43b81912b,

title = "Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes",

abstract = "All-solid-state lithium batteries (ASSLBs) with nonflammable solid electrolytes (SEs) deliver greatly enhanced safety characteristics. Furthermore, ASSLBs composed of cathodes with high working voltages, such as LiCoO2, LiNixCoyMnzO2 (x + y + z = 1, NCM), LiNixCoyAlzO2 (x + y + z = 1, NCA), LiMnxFeyPO4 (x + y = 1, LMFP), and LiNi0.5Mn1.5O4 (LNMO), and a lithium metal anode can achieve comparable or better performance compared with that of LLBs in terms of energy density. Therefore, high-voltage ASSLBs have been regarded as the most promising next-generation batteries. Although significant progress has been achieved in high-voltage ASSLBs research, their development still faces multiple challenges. To facilitate further effective and target-oriented research on high-voltage ASSLBs, a summary of recent research progress is urgently needed. In this review, recent research progress in high-voltage ASSLBs is summarized from the perspectives of SEs modification, interfacial challenges and their corresponding solutions for cathodes, and high-voltage composite cathode design for practical applications. Finally, the authors{\textquoteright} perspectives on the state of current ASSLBs research, aiming to propose possible research directions for the future development of high-voltage ASSLBs.",

keywords = "high energy density, high-voltage cathodes, lithium batteries, solid-state batteries",

author = "Liansheng Li and Huanhuan Duan and Jia Li and Lei Zhang and Yuanfu Deng and Guohua Chen",

note = "Funding Information: This work was supported by the National Natural Science Foundation of China (Grant No. 21875071, 51621001), the National Natural Science Foundation of China–Hong Kong Research Grant Council (NSFC‐RGC) Joint Research Scheme (Grant No. 21661162002 and N_HKUST601/16) and R&D Projects in Key Areas of Guangdong Province (2019B090908001). The authors thank Huifang Fei and Huawen Huang for language editing and revision of the manuscript. Funding Information: This work was supported by the National Natural Science Foundation of China (Grant No. 21875071, 51621001), the National Natural Science Foundation of China?Hong Kong Research Grant Council (NSFC-RGC) Joint Research Scheme (Grant No. 21661162002 and N_HKUST601/16) and R&D Projects in Key Areas of Guangdong Province (2019B090908001). The authors thank Huifang Fei and Huawen Huang for language editing and revision of the manuscript. Publisher Copyright: {\textcopyright} 2021 Wiley-VCH GmbH",

year = "2021",

month = jul,

day = "28",

doi = "10.1002/aenm.202003154",

language = "English",

volume = "11",

journal = "Advanced Energy Materials",

issn = "1614-6832",

publisher = "Wiley-VCH Verlag",

number = "28",

}

Li, L, Duan, H, Li, J, Zhang, L, Deng, Y & Chen, G 2021, 'Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes', Advanced Energy Materials, vol. 11, no. 28, 2003154. https://doi.org/10.1002/aenm.202003154

Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes. / Li, Liansheng; Duan, Huanhuan; Li, Jia et al.
In: Advanced Energy Materials, Vol. 11, No. 28, 2003154, 28.07.2021.

Research output: Journal article publication › Review article › Academic research › peer-review

TY - JOUR

T1 - Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes

AU - Li, Liansheng

AU - Duan, Huanhuan

AU - Li, Jia

AU - Zhang, Lei

AU - Deng, Yuanfu

AU - Chen, Guohua

N1 - Funding Information:This work was supported by the National Natural Science Foundation of China (Grant No. 21875071, 51621001), the National Natural Science Foundation of China–Hong Kong Research Grant Council (NSFC‐RGC) Joint Research Scheme (Grant No. 21661162002 and N_HKUST601/16) and R&D Projects in Key Areas of Guangdong Province (2019B090908001). The authors thank Huifang Fei and Huawen Huang for language editing and revision of the manuscript.Funding Information:This work was supported by the National Natural Science Foundation of China (Grant No. 21875071, 51621001), the National Natural Science Foundation of China?Hong Kong Research Grant Council (NSFC-RGC) Joint Research Scheme (Grant No. 21661162002 and N_HKUST601/16) and R&D Projects in Key Areas of Guangdong Province (2019B090908001). The authors thank Huifang Fei and Huawen Huang for language editing and revision of the manuscript.Publisher Copyright:© 2021 Wiley-VCH GmbH

PY - 2021/7/28

Y1 - 2021/7/28

N2 - All-solid-state lithium batteries (ASSLBs) with nonflammable solid electrolytes (SEs) deliver greatly enhanced safety characteristics. Furthermore, ASSLBs composed of cathodes with high working voltages, such as LiCoO2, LiNixCoyMnzO2 (x + y + z = 1, NCM), LiNixCoyAlzO2 (x + y + z = 1, NCA), LiMnxFeyPO4 (x + y = 1, LMFP), and LiNi0.5Mn1.5O4 (LNMO), and a lithium metal anode can achieve comparable or better performance compared with that of LLBs in terms of energy density. Therefore, high-voltage ASSLBs have been regarded as the most promising next-generation batteries. Although significant progress has been achieved in high-voltage ASSLBs research, their development still faces multiple challenges. To facilitate further effective and target-oriented research on high-voltage ASSLBs, a summary of recent research progress is urgently needed. In this review, recent research progress in high-voltage ASSLBs is summarized from the perspectives of SEs modification, interfacial challenges and their corresponding solutions for cathodes, and high-voltage composite cathode design for practical applications. Finally, the authors’ perspectives on the state of current ASSLBs research, aiming to propose possible research directions for the future development of high-voltage ASSLBs.

AB - All-solid-state lithium batteries (ASSLBs) with nonflammable solid electrolytes (SEs) deliver greatly enhanced safety characteristics. Furthermore, ASSLBs composed of cathodes with high working voltages, such as LiCoO2, LiNixCoyMnzO2 (x + y + z = 1, NCM), LiNixCoyAlzO2 (x + y + z = 1, NCA), LiMnxFeyPO4 (x + y = 1, LMFP), and LiNi0.5Mn1.5O4 (LNMO), and a lithium metal anode can achieve comparable or better performance compared with that of LLBs in terms of energy density. Therefore, high-voltage ASSLBs have been regarded as the most promising next-generation batteries. Although significant progress has been achieved in high-voltage ASSLBs research, their development still faces multiple challenges. To facilitate further effective and target-oriented research on high-voltage ASSLBs, a summary of recent research progress is urgently needed. In this review, recent research progress in high-voltage ASSLBs is summarized from the perspectives of SEs modification, interfacial challenges and their corresponding solutions for cathodes, and high-voltage composite cathode design for practical applications. Finally, the authors’ perspectives on the state of current ASSLBs research, aiming to propose possible research directions for the future development of high-voltage ASSLBs.

KW - high energy density

KW - high-voltage cathodes

KW - lithium batteries

KW - solid-state batteries

UR - http://www.scopus.com/inward/record.url?scp=85107344740&partnerID=8YFLogxK

U2 - 10.1002/aenm.202003154

DO - 10.1002/aenm.202003154

M3 - Review article

SN - 1614-6832

VL - 11

JO - Advanced Energy Materials

JF - Advanced Energy Materials

IS - 28

M1 - 2003154

ER -

Li L, Duan H, Li J, Zhang L, Deng Y, Chen G. Toward High Performance All-Solid-State Lithium Batteries with High-Voltage Cathode Materials: Design Strategies for Solid Electrolytes, Cathode Interfaces, and Composite Electrodes. Advanced Energy Materials. 2021 Jul 28;11(28):2003154. Epub 2021 Jun 9. doi: 10.1002/aenm.202003154